Experimental confirmation of a new paradigm of spin exchange in dilute solutions of paramagnetic particles

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Resumo

The new paradigm of spin exchange and its manifestations in EPR spectroscopy contain provisions that are fundamentally different from the widespread initial paradigm of spin exchange. The new paradigm of spin exchange in dilute solutions is also of interest as an example of the formation of a coordinated spin coherence motion of an ensemble of spins in a dilute paramagnetic, and this consistency is achieved by random bimolecular collisions of paramagnetic particles, in fact, the «recoil effect» of spin coherence in random collisions of paramagnetic particles. The new paradigm of spin exchange and new protocols for analyzing experimental data will be more widely recognized and used as a tool, for example, to improve the accuracy of detecting the frequency of collisions of substrate molecules with receptors in molecular biology using EPR spectroscopy. The experimental evidence of the fundamental provisions of the new paradigm obtained in the last 2–3 years are discussed.

Sobre autores

K. Salikhov

Zavoisky Physical-Technical Institute, Federal Research Center Kazan Scientific Center of the Russian Academy of Sciences

Email: kevsalikhov@mail.ru
Kazan, Russia

Bibliografia

  1. Замараев К.И., Молин Ю.Н., Салихов К.М. Спиновый обмен. Новосибирск: Наука. Сибир. отд., 1977.
  2. Molin Yu.N., Salikhov K.M., and Zamaraev K.I. Spin exchange. Application in chemistry and biology. Berlin: Springer Verlag, 1980.
  3. Bales B.L. // in: Biological magnetic resonance. V. 8. P. 77. N.Y.: Plenum Publishing Corporation, 1989.
  4. Салихов К.М. // УФН. 2019. Т. 189. С. 1017
  5. Salikhov K.M. Fundamentals of spin exchange. Story of paradigm shift. Cham: Springer Nature, 2019.
  6. Salikhov K.M. // Appl. Magn. Reson. 2020. V. 51. P. 297.
  7. Salikhov K.M. // Appl. Magn. Reson. 2025. V. 56. No. 1.
  8. Salikhov K.M. // J. Magn. Reson. 1985. V. 63. P. 271.
  9. Салихов К.М. // Изв. РАН. Сер. физ. 2020. Т. 84. С. 659
  10. Галеев Р.Т., Салихов К.М. // Хим. физика. 1996. Т. 15. С. 48
  11. Salikhov K.M. // J. Magn. Reson. 1985. V. 63. P. 271.
  12. Salikhov K.M. // Appl. Magn. Reson. 2010. V. 38. P. 237.
  13. Salikhov K.M. // Appl. Magn. Reson. 2016. V. 47. P. 1207.
  14. Bales B.L., Bakirov M.M., Galeev R.T. et al. // Appl. Magn. Reson. 2017. V. 48. P. 1399.
  15. Salikhov K.M. // Appl. Magn. Reson. 2018. V. 49. P. 1417.
  16. Salikhov K.M. // J. Phys. Chem. B. 2020. V. 124. P. 6628.
  17. Salikhov K.M. // Appl. Magn. Reson. 2021. V. 52. P. 1063.
  18. Bakirov M.M., Khairutdinov I.T., Salikhov K.M. et al. // Appl. Magn. Reson. 2022. V. 53. P. 1275.
  19. Salikhov K.M., Bakirov M.M., Khairutdinov I.T., and Zaripov R.B. // J. Magn. Reson. 2024. V. 363. P. 107703.
  20. Bales B.L., Peric M., and Schwartz R.N. // J. Phys. Chem. Lett. 2024. V. 15. P. 2082.
  21. Solomon I. // Phys. Rev. 1955. V. 99. P. 559.
  22. Абрагам А. Ядерный магнетизм. М.: ИЛ, 1963.
  23. Салихов К.М., Семенов А.Г., Цветков Ю.Д. Электронное спиновое эхо и его применение. Новосибирск: Наука. Сибир. отд., 1976.
  24. Bakirov M.M., Khairutdinov I.T., Zaripov R.B., and Salikhov K.M. // Book abstr. MDMR-24 (Kazan, 2024). P. 134.
  25. Wolf E.L. // Phys. Rev. 1966. V. 142. P. 555.
  26. Marsh D. // J. Magn. Reson. 2017. V. 277. P. 86.
  27. Salikhov K.M., Bakirov M.M., Zaripov R.B., and Khairutdinov I.T. // Phys. Chem. Chem. Phys. 2023. V. 25. P. 17966.
  28. Bales B.L., Peric M., Dragutan I. et al. // J. Phys. Chem. Lett. 2022. V. 13. P. 10952.
  29. Салихов К.М. // ЖЭТФ. 2022. Т. 162. С. 630

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